@article{Ye_Jiang_Li_Wu_Chen_2021, title={Rational Design of MOF-Based Materials for Next-Generation Rechargeable Batteries}, volume={13}, url={https://nmlett.org/index.php/nml/article/view/970}, DOI={10.1007/s40820-021-00726-z}, abstractNote={<p>Metal–organic framework (MOF)-based materials with high porosity, tunable compositions, diverse structures, and versatile functionalities provide great scope for next-generation rechargeable battery applications. Herein, this review summarizes recent advances in pristine MOFs, MOF composites, MOF derivatives, and MOF composite derivatives for high-performance sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, lithium–sulfur batteries, lithium–oxygen batteries, and Zn–air batteries in which the unique roles of MOFs as electrodes, separators, and even electrolyte are highlighted. Furthermore, through the discussion of MOF-based materials in each battery system, the key principles for controllable synthesis of diverse MOF-based materials and electrochemical performance improvement mechanisms are discussed in detail. Finally, the major challenges and perspectives of MOFs are also proposed for next-generation battery applications.</p> <p>Highlights:</p> <p>1 This review summarizes recent progresses in pristine metal–organic frameworks (MOFs), MOF composites, and their derivatives for next-generation rechargeable batteries including lithium–sulfur batteries, lithium–oxygen batteries, sodium-ion batteries, potassium-ion batteries, Zn-ion batteries, and Zn–air batteries.<br>2 The design strategies for MOF-based materials as the electrode, separator, and electrolyte are outlined and discussed.<br>3 The challenges and development strategies and of MOF-related materials for battery applications are highlighted.</p>}, journal={Nano-Micro Letters}, author={Ye, Zhengqing and Jiang, Ying and Li, Li and Wu, Feng and Chen, Renjie}, year={2021}, month={Oct.}, pages={203} }