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Vol. 15 (2023)

A General Strategy for Ordered Carrier Transport of Quasi-2D and 3D Perovskite Films for Giant Self-Powered Photoresponse and Ultrahigh Stability

https://doi.org/10.1007/s40820-023-01087-5
Fei Zhu
State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, People’s Republic of China
Gang Lian
State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, People’s Republic of China
Deliang Cui
State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, People’s Republic of China
Qilong Wang
Key Laboratory for Special Functional Aggregated Materials of Education Ministry, School of Chemistry & Chemical Engineering, Shandong University, Jinan 250100, People’s Republic of China
Haohai Yu
State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, People’s Republic of China
Huaijin Zhang
State Key Laboratory of Crystal Materials, Shandong University, Jinan 250100, People’s Republic of China
Qingbo Meng
Key Laboratory for Renewable Energy, Chinese Academy of Sciences (CAS), Beijing, People’s Republic of China
Ching‑Ping Wong
School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA 30332, USA

Corresponding Author: Ching‑Ping Wong

cp.wong@mse.gatech.edu

Nano-Micro Letters, Vol. 15 (2023), Article Number: 115

Abstract

Organic–inorganic hybrid perovskite materials have been focusing more attention in the field of self-powered photodetectors due to their superb photoelectric properties. However, a universal growth approach is required and challenging to realize vertically oriented growth and grain boundary fusion of 2D and 3D perovskite grains to promote ordered carrier transport, which determines superior photoresponse and high stability. Herein, a general thermal-pressed (TP) strategy is designed to solve the above issues, achieving uniaxial orientation and single-grain penetration along the film thickness direction. It constructs the efficient channel for ordered carrier transport between two electrodes. Combining of the improved crystal quality and lower trap-state density, the quasi-2D and 3D perovskite-based self-powered photodetector devices (with/without hole transport layer) all exhibit giant and stable photoresponse in a wide spectrum range and specific wavelength laser. For the MAPbI3-based self-powered photodetectors, the largest Rλ value is as high as 0.57 A W−1 at 760 nm, which is larger than most reported results. Meanwhile, under laser illumination (532 nm), the FPEA2MA4Pb5I16-based device exhibits a high responsivity (0.4 A W−1) value, which is one of the best results in 2DRP self-powered photodetectors. In addition, fast response, ultralow detection limit, and markedly improved humidity, optical and heat stabilities are clearly demonstrated for these TP-based devices.


Highlights:


1 Uniaxial orientation and single-grain penetration of quasi-2D and 3D perovskite films were achieved via a general thermal-pressed (TP) strategy.
2 The TP-perovskite-based self-powered photodetectors (SPPDs) exhibit one of the best results among the 3D and quasi-2D perovskite SPPDs, respectively.
3 These unpackaged TP-based devices exhibit ultrahigh humidity, optical and heat stability.

Keywords

Perovskites Thermal-pressed strategy Uniaxial orientation Self-powered photodetectors Stability
Zhu, Fei, Gang Lian, Deliang Cui, Qilong Wang, Haohai Yu, Huaijin Zhang, Qingbo Meng, and Ching‑Ping Wong. 2023. “A General Strategy for Ordered Carrier Transport of Quasi-2D and 3D Perovskite Films for Giant Self-Powered Photoresponse and Ultrahigh Stability”. Nano-Micro Letters 15 (April):115. https://doi.org/10.1007/s40820-023-01087-5.
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