Issue

Vol. 14 (2022)

Layered Foam/Film Polymer Nanocomposites with Highly Efficient EMI Shielding Properties and Ultralow Reflection

https://doi.org/10.1007/s40820-021-00759-4
Li Ma
Department of Mechanical and Industrial Engineering, University of Toronto, 5 King’s College Road, Toronto, ON M5S 3G8, Canada
Mahdi Hamidinejad
Department of Mechanical and Industrial Engineering, University of Toronto, 5 King’s College Road, Toronto, ON M5S 3G8, Canada
Biao Zhao
Department of Mechanical and Industrial Engineering, University of Toronto, 5 King’s College Road, Toronto, ON M5S 3G8, Canada
Caiyun Liang
Department of Mechanical and Industrial Engineering, University of Toronto, 5 King’s College Road, Toronto, ON M5S 3G8, Canada
Chul B. Park
Department of Mechanical and Industrial Engineering, University of Toronto, 5 King’s College Road, Toronto, ON M5S 3G8, Canada

Corresponding Author: Chul B. Park

park@mie.utoronto.ca

Nano-Micro Letters, Vol. 14 (2022), Article Number: 19

Abstract

Lightweight, high-efficiency and low reflection electromagnetic interference (EMI) shielding polymer composites are greatly desired for addressing the challenge of ever-increasing electromagnetic pollution. Lightweight layered foam/film PVDF nanocomposites with efficient EMI shielding effectiveness and ultralow reflection power were fabricated by physical foaming. The unique layered foam/film structure was composed of PVDF/SiCnw/MXene (Ti3C2Tx) composite foam as absorption layer and highly conductive PVDF/MWCNT/GnPs composite film as a reflection layer. The foam layer with numerous heterogeneous interfaces developed between the SiC nanowires (SiCnw) and 2D MXene nanosheets imparted superior EM wave attenuation capability. Furthermore, the microcellular structure effectively tuned the impedance matching and prolonged the wave propagating path by internal scattering and multiple reflections. Meanwhile, the highly conductive PVDF/MWCNT/GnPs composite (~ 220 S m−1) exhibited superior reflectivity (R) of 0.95. The tailored structure in the layered foam/film PVDF nanocomposite exhibited an EMI SE of 32.6 dB and a low reflection bandwidth of 4 GHz (R < 0.1) over the Ku-band (12.4 − 18.0 GHz) at a thickness of 1.95 mm. A peak SER of 3.1 × 10–4 dB was obtained which corresponds to only 0.0022% reflection efficiency. In consequence, this study introduces a feasible approach to develop lightweight, high-efficiency EMI shielding materials with ultralow reflection for emerging applications.


Highlights:


1 The successful fabrication of layered foam/film structure via the crystal melting temperature mismatch for two grades of PVDF resin in a batch foaming process.
2 Developing the heterostructure interfaces between SiC nanowires and MXene (Ti3C2Tx) nanosheets.
3 Achieving efficient electromagnetic interference shielding effectiveness with ultralow reflectivity.

Keywords

2D MXene nanosheets SiC nanowires Layered foam/film polymer nanocomposites Microcellular structure Absorption-dominated EMI shielding
Ma, Li, Mahdi Hamidinejad, Biao Zhao, Caiyun Liang, and Chul B. Park. 2021. “Layered Foam/Film Polymer Nanocomposites With Highly Efficient EMI Shielding Properties and Ultralow Reflection”. Nano-Micro Letters 14 (December):19. https://doi.org/10.1007/s40820-021-00759-4.
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