Issue

Vol. 15 (2023)

Advances in Mn-Based Electrode Materials for Aqueous Sodium-Ion Batteries

https://doi.org/10.1007/s40820-023-01162-x
Changsheng Ding
School of Materials Science and Engineering, Shanghai University, Shanghai 200444, People’s Republic of China
Zhang Chen
School of Materials Science and Engineering, Shanghai University, Shanghai 200444, People’s Republic of China
Chuanxiang Cao
School of Materials Science and Engineering, Shanghai University, Shanghai 200444, People’s Republic of China
Yu Liu
Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, People’s Republic of China
Yanfeng Gao
School of Materials Science and Engineering, Shanghai University, Shanghai 200444, People’s Republic of China

Corresponding Author: Yanfeng Gao

yfgao@shu.edu.cn

Nano-Micro Letters, Vol. 15 (2023), Article Number: 192

Abstract

Aqueous sodium-ion batteries have attracted extensive attention for large-scale energy storage applications, due to abundant sodium resources, low cost, intrinsic safety of aqueous electrolytes and eco-friendliness. The electrochemical performance of aqueous sodium-ion batteries is affected by the properties of electrode materials and electrolytes. Among various electrode materials, Mn-based electrode materials have attracted tremendous attention because of the abundance of Mn, low cost, nontoxicity, eco-friendliness and interesting electrochemical performance. Aqueous electrolytes having narrow electrochemical window also affect the electrochemical performance of Mn-based electrode materials. In this review, we introduce systematically Mn-based electrode materials for aqueous sodium-ion batteries from cathode and anode materials and offer a comprehensive overview about their recent development. These Mn-based materials include oxides, Prussian blue analogues and polyanion compounds. We summarize and discuss the composition, crystal structure, morphology and electrochemical properties of Mn-based electrode materials. The improvement methods based on electrolyte optimization, element doping or substitution, optimization of morphology and carbon modification are highlighted. The perspectives of Mn-based electrode materials for future studies are also provided. We believe this review is important and helpful to explore and apply Mn-based electrode materials in aqueous sodium-ion batteries.


Highlights:
1 Mn-based electrode materials, including oxides, Prussian blue analogues and polyanion compounds, are introduced systematically for aqueous sodium-ion batteries.
2 The composition, crystal structure, morphology and electrochemical performance of Mn-based electrode materials are reviewed.
3 The improvement methods of electrochemical performance, such as electrolyte optimization, element doping or substitution, morphology optimization and carbon modification, are discussed.

Keywords

Sodium-ion batteries Aqueous electrolytes Mn-based electrode materials Electrochemical performance Improvement methods
Ding, Changsheng, Zhang Chen, Chuanxiang Cao, Yu Liu, and Yanfeng Gao. 2023. “Advances in Mn-Based Electrode Materials for Aqueous Sodium-Ion Batteries”. Nano-Micro Letters 15 (August):192. https://doi.org/10.1007/s40820-023-01162-x.
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