Issue

Vol. 15 (2023)

Integration of Multiple Heterointerfaces in a Hierarchical 0D@2D@1D Structure for Lightweight, Flexible, and Hydrophobic Multifunctional Electromagnetic Protective Fabrics

https://doi.org/10.1007/s40820-023-01179-2
Shuo Zhang
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑Fibers and Eco‑Textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Xuehua Liu
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑Fibers and Eco‑Textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Chenyu Jia
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑Fibers and Eco‑Textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Zhengshuo Sun
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑Fibers and Eco‑Textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Haowen Jiang
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑Fibers and Eco‑Textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Zirui Jia
College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Guanglei Wu
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑Fibers and Eco‑Textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China

Corresponding Author: Guanglei Wu

wuguanglei@qdu.edu.cn

Nano-Micro Letters, Vol. 15 (2023), Article Number: 204

Abstract

The development of wearable multifunctional electromagnetic protective fabrics with multifunctional, low cost, and high efficiency remains a challenge. Here, inspired by the unique flower branch shape of “Thunberg’s meadowsweet” in nature, a nanofibrous composite membrane with hierarchical structure was constructed. Integrating sophisticated 0D@2D@1D hierarchical structures with multiple heterointerfaces can fully unleash the multifunctional application potential of composite membrane. The targeted induction method was used to precisely regulate the formation site and morphology of the metal–organic framework precursor, and intelligently integrate multiple heterostructures to enhance dielectric polarization, which improves the impedance matching and loss mechanisms of the electromagnetic wave absorbing materials. Due to the synergistic enhancement of electrospinning-derived carbon nanofiber “stems”, MOF-derived carbon nanosheet “petals” and transition metal selenide nano-particle “stamens”, the CoxSey/NiSe@CNSs@CNFs (CNCC) composite membrane obtains a minimum reflection loss value (RLmin) of -68.40 dB at 2.6 mm and a maximum effective absorption bandwidth (EAB) of 8.88 GHz at a thin thickness of 2.0 mm with a filling amount of only 5 wt%. In addition, the multi-component and hierarchical heterostructure endow the fibrous membrane with excellent flexibility, water resistance, thermal management, and other multifunctional properties. This work provides unique perspectives for the precise design and rational application of multifunctional fabrics.


Highlights:
1 Electrospinning combined with structural engineering to construct 0D@2D@1D hierarchical heterogeneous interfaces.
2 A “mechanical response” model was constructed to explain the stress transfer mechanism of fibrous membranes with 2D@1D structures.
3 The “One for All” fibrous membrane combines excellent flexibility, mechanical properties, waterproof, and electromagnetic protection.

Keywords

Electrostatic spinning MOFs Bimetallic selenide Hierarchical structures Multiple heterointerfaces Electromagnetic wave absorption
Zhang, Shuo, Xuehua Liu, Chenyu Jia, Zhengshuo Sun, Haowen Jiang, Zirui Jia, and Guanglei Wu. 2023. “Integration of Multiple Heterointerfaces in a Hierarchical 0D@2D@1D Structure for Lightweight, Flexible, and Hydrophobic Multifunctional Electromagnetic Protective Fabrics”. Nano-Micro Letters 15 (August):204. https://doi.org/10.1007/s40820-023-01179-2.
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