Issue

Vol. 15 (2023)

Construction of Self-Assembly Based Tunable Absorber: Lightweight, Hydrophobic and Self-Cleaning Properties

https://doi.org/10.1007/s40820-023-01108-3
Zehua Zhou
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑fibers and Eco‑textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Qianqian Zhu
College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Yue Liu
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑fibers and Eco‑textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Yan Zhang
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑fibers and Eco‑textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Zirui Jia
College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, People’s Republic of China
Guanglei Wu
Institute of Materials for Energy and Environment, State Key Laboratory of Bio‑fibers and Eco‑textiles, College of Materials Science and Engineering, Qingdao University, Qingdao 266071, People’s Republic of China

Corresponding Author: Guanglei Wu

wuguanglei@qdu.edu.cn

Nano-Micro Letters, Vol. 15 (2023), Article Number: 137

Abstract

Although multifunctional aerogels are expected to be used in applications such as portable electronic devices, it is still a great challenge to confer multifunctionality to aerogels while maintaining their inherent microstructure. Herein, a simple method is proposed to prepare multifunctional NiCo/C aerogels with excellent electromagnetic wave absorption properties, superhydrophobicity, and self-cleaning by water-induced NiCo-MOF self-assembly. Specifically, the impedance matching of the three-dimensional (3D) structure and the interfacial polarization provided by CoNi/C as well as the defect-induced dipole polarization are the primary contributors to the broadband absorption. As a result, the prepared NiCo/C aerogels have a broadband width of 6.22 GHz at 1.9 mm. Due to the presence of hydrophobic functional groups, CoNi/C aerogels improve the stability in humid environments and obtain hydrophobicity with large contact angles > 140°. This multifunctional aerogel has promising applications in electromagnetic wave absorption, resistance to water or humid environments.


Highlights:


1 NiCo/C aerogel was prepared by pyrolysis carbonization self-assembly of NiCo- metal–organic frameworks (MOFs).
2 The assembly mechanism of MOF aerogel was studied by adjusting the ratio of metal ion /BTC.
3 Aerogel combines hydrophobic, lightweight, self-cleaning, and electromagnetic wave absorption properties.

Keywords

MOF aerogel Self-cleaning Electromagnetic wave absorption Hydrophobic
Zhou, Zehua, Qianqian Zhu, Yue Liu, Yan Zhang, Zirui Jia, and Guanglei Wu. 2023. “Construction of Self-Assembly Based Tunable Absorber: Lightweight, Hydrophobic and Self-Cleaning Properties”. Nano-Micro Letters 15 (May):137. https://doi.org/10.1007/s40820-023-01108-3.
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