Issue

Vol. 16 (2024)

MXene Hollow Spheres Supported by a C–Co Exoskeleton Grow MWCNTs for Efficient Microwave Absorption

https://doi.org/10.1007/s40820-024-01326-3
Ze Wu
School of Mechanical Engineering, Southeast University, Nanjing 211189, People’s Republic of China
Xiuli Tan
School of Mechanical Engineering, Southeast University, Nanjing 211189, People’s Republic of China
Jianqiao Wang
School of Mechanical Engineering, Southeast University, Nanjing 211189, People’s Republic of China
Youqiang Xing
School of Mechanical Engineering, Southeast University, Nanjing 211189, People’s Republic of China
Peng Huang
School of Mechanical Engineering, Southeast University, Nanjing 211189, People’s Republic of China
Bingjue Li
School of Mechanical Engineering, Southeast University, Nanjing 211189, People’s Republic of China
Lei Liu
School of Mechanical Engineering, Southeast University, Nanjing 211189, People’s Republic of China

Corresponding Author: Lei Liu

liulei@seu.edu.cn

Nano-Micro Letters, Vol. 16 (2024), Article Number: 107

Abstract

High-performance microwave absorption (MA) materials must be studied immediately since electromagnetic pollution has become a problem that cannot be disregarded. A straightforward composite material, comprising hollow MXene spheres loaded with C–Co frameworks, was prepared to develop multiwalled carbon nanotubes (MWCNTs). A high impedance and suitable morphology were guaranteed by the C–Co exoskeleton, the attenuation ability was provided by the MWCNTs endoskeleton, and the material performance was greatly enhanced by the layered core–shell structure. When the thickness was only 2.04 mm, the effective absorption bandwidth was 5.67 GHz, and the minimum reflection loss (RLmin) was − 70.70 dB. At a thickness of 1.861 mm, the sample calcined at 700 °C had a RLmin of − 63.25 dB. All samples performed well with a reduced filler ratio of 15 wt%. This paper provides a method for making lightweight core–shell composite MA materials with magnetoelectric synergy.


Highlights:
1 A hollow core–shell structure was constructed with C–Co as the exoskeleton to support the MXene and multiwalled carbon nanotubes (MWCNTs) endoskeleton, with MWCNTs growing toward the center of the sphere.
2 A reflection loss of − 70.70 dB and an effective absorption bandwidth of 5.67 GHz were obtained when the thickness was only 2.04 mm. The powder filler ratio was only 15 wt%.
3 The unique hollow core–shell structure enhanced multiple reflection and scattering losses.

Keywords

MXene C–Co skeleton MWCNTs Microwave absorption
Wu, Ze, Xiuli Tan, Jianqiao Wang, Youqiang Xing, Peng Huang, Bingjue Li, and Lei Liu. 2024. “MXene Hollow Spheres Supported by a C–Co Exoskeleton Grow MWCNTs for Efficient Microwave Absorption”. Nano-Micro Letters 16 (February):107. https://doi.org/10.1007/s40820-024-01326-3.
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