Issue

Vol. 17 (2025)

Yolk–Shell CoNi@N-Doped Carbon-CoNi@CNTs for Enhanced Microwave Absorption, Photothermal, Anti-Corrosion, and Antimicrobial Properties

https://doi.org/10.1007/s40820-024-01626-8
Qiqin Liang
College of Physics, Guizhou Province Key Laboratory for Photoelectrics Technology and Application, Guizhou University, Guiyang City 550025, People’s Republic of China
Mukun He
Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Beibei Zhan
College of Physics, Guizhou Province Key Laboratory for Photoelectrics Technology and Application, Guizhou University, Guiyang City 550025, People’s Republic of China
Hua Guo
Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China
Xiaosi Qi
College of Physics, Guizhou Province Key Laboratory for Photoelectrics Technology and Application, Guizhou University, Guiyang City 550025, People’s Republic of China
Yunpeng Qu
College of Physics, Guizhou Province Key Laboratory for Photoelectrics Technology and Application, Guizhou University, Guiyang City 550025, People’s Republic of China
Yali Zhang
College of Physics, Guizhou Province Key Laboratory for Photoelectrics Technology and Application, Guizhou University, Guiyang City 550025, People’s Republic of China
Wei Zhong
National Laboratory of Solid State Microstructures and Jiangsu Provincial Laboratory for NanoTechnology, Nanjing University, Nanjing 210093, People’s Republic of China
Junwei Gu
Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an 710072, People’s Republic of China

Corresponding Author: Junwei Gu

gjw@nwpu.edu.cn

Nano-Micro Letters, Vol. 17 (2025), Article Number: 167

Abstract

The previous studies mainly focused on improving microwave absorbing (MA) performances of MA materials. Even so, these designed MA materials were very difficult to be employed in complex and changing environments owing to their single-functionalities. Herein, a combined Prussian blue analogues derived and catalytical chemical vapor deposition strategy was proposed to produce hierarchical cubic sea urchin-like yolk–shell CoNi@N-doped carbon (NC)-CoNi@carbon nanotubes (CNTs) mixed-dimensional multicomponent nanocomposites (MCNCs), which were composed of zero-dimensional CoNi nanoparticles, three-dimensional NC nanocubes and one-dimensional CNTs. Because of good impedance matching and attenuation characteristics, the designed CoNi@NC-CoNi@CNTs mixed-dimensional MCNCs exhibited excellent MA performances, which achieved a minimum reflection loss (RLmin) of −71.70 dB at 2.78 mm and Radar Cross section value of −53.23 dB m2. More importantly, the acquired results demonstrated that CoNi@NC-CoNi@CNTs MCNCs presented excellent photothermal, antimicrobial and anti-corrosion properties owing to their hierarchical cubic sea urchin-like yolk–shell structure, highlighting their potential multifunctional applications. It could be seen that this finding not only presented a generalizable route to produce hierarchical cubic sea urchin-like yolk–shell magnetic NC-CNTs-based mixed-dimensional MCNCs, but also provided an effective strategy to develop multifunctional MCNCs and improve their environmental adaptabilities.


Highlights:
1 Hierarchical cubic sea urchin-like yolk-shell CoNi@N-doped carbon (NC)-CoNi@carbon nanotubes (CNTs) mixed-dimensional MCNCs with different CNTs contents could be availably and selectively synthesized.
2 Owing to the generated hierarchical cubic sea urchin like yolk-shell structure, CoNi@NC-CoNi@CNTs display marvelous hydrophobic, corrosion resistance and MA performance.
3 The construction of components and special microstructure make CoNi@NC-CoNi@CNTs MCNCs display terrific photothermal and antimicrobial (e g. only 1 mg·mL-1 concentration, ~84.03% antimicrobial rate) proper ties.

Keywords

Sea urchin Like yolk Shell structure CoNi@N Doped carbon CoNi@carbon nanotubes Mixed Dimensional nanocomposites Microwave absorption Photothermal and antimicrobial
Liang, Qiqin, Mukun He, Beibei Zhan, Hua Guo, Xiaosi Qi, Yunpeng Qu, Yali Zhang, Wei Zhong, and Junwei Gu. 2025. “Yolk–Shell CoNi@N-Doped Carbon-CoNi@CNTs for Enhanced Microwave Absorption, Photothermal, Anti-Corrosion, and Antimicrobial Properties”. Nano-Micro Letters 17 (February):167. https://doi.org/10.1007/s40820-024-01626-8.
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