Issue

Vol. 12 (2020)

High-Performance Aqueous Zinc-Ion Batteries Realized by MOF Materials

https://doi.org/10.1007/s40820-020-00487-1
Xuechao Pu
Shenzhen Geim Graphene Center, Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen 518055, People’s Republic of China
Baozheng Jiang
Shenzhen Geim Graphene Center, Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen 518055, People’s Republic of China
Xianli Wang
Shenzhen Geim Graphene Center, Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen 518055, People’s Republic of China
Wenbao Liu
Shenzhen Geim Graphene Center, Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen 518055, People’s Republic of China
Liubing Dong
College of Chemistry and Materials Science, Jinan University, Guangzhou 511443, People’s Republic of China
Feiyu Kang
Shenzhen Geim Graphene Center, Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen 518055, People’s Republic of China
Chengjun Xu
Shenzhen Geim Graphene Center, Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen 518055, People’s Republic of China

Corresponding Author: Chengjun Xu

vivaxuchengjun@163.com

Nano-Micro Letters, Vol. 12 (2020), Article Number: 152

Abstract

Rechargeable aqueous zinc-ion batteries (ZIBs) have been gaining increasing interest for large-scale energy storage applications due to their high safety, good rate capability, and low cost. However, the further development of ZIBs is impeded by two main challenges: Currently reported cathode materials usually suffer from rapid capacity fading or high toxicity, and meanwhile, unstable zinc stripping/plating on Zn anode seriously shortens the cycling life of ZIBs. In this paper, metal–organic framework (MOF) materials are proposed to simultaneously address these issues and realize high-performance ZIBs with Mn(BTC) MOF cathodes and ZIF-8-coated Zn (ZIF-8@Zn) anodes. Various MOF materials were synthesized, and Mn(BTC) MOF was found to exhibit the best Zn2+-storage ability with a capacity of 112 mAh g−1. Zn2+ storage mechanism of the Mn(BTC) was carefully studied. Besides, ZIF-8@Zn anodes were prepared by coating ZIF-8 MOF material on Zn foils. Unique porous structure of the ZIF-8 coating guided uniform Zn stripping/plating on the surface of Zn anodes. As a result, the ZIF-8@Zn anodes exhibited stable Zn stripping/plating behaviors, with 8 times longer cycle life than bare Zn foils. Based on the above, high-performance aqueous ZIBs were constructed using the Mn(BTC) cathodes and the ZIF-8@Zn anodes, which displayed an excellent long-cycling stability without obvious capacity fading after 900 charge/discharge cycles. This work provides a new opportunity for high-performance energy storage system.


Highlights:


1 Various MOF materials were synthesized and investigated as ZIB cathodes.
2 A long-term stable ZIF-8@Zn anode was proposed by coating ZIF-8 material on the surface of zinc foils.
3 High-performance aqueous ZIBs were constructed using the Mn(BTC) cathode and the ZIF-8@Zn anode.

Keywords

Zinc-ion battery Metal–organic framework Cathode material Zn anode
Pu, Xuechao, Baozheng Jiang, Xianli Wang, Wenbao Liu, Liubing Dong, Feiyu Kang, and Chengjun Xu. 2020. “High-Performance Aqueous Zinc-Ion Batteries Realized by MOF Materials”. Nano-Micro Letters 12 (July):152. https://doi.org/10.1007/s40820-020-00487-1.
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