Issue

Vol. 16 (2024)

Leakage Proof, Flame-Retardant, and Electromagnetic Shield Wood Morphology Genetic Composite Phase Change Materials for Solar Thermal Energy Harvesting

https://doi.org/10.1007/s40820-024-01414-4
Yuhui Chen
Yunnan Provincial Key Laboratory of Energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials, The International Joint Laboratory for Sustainable Polymers of Yunnan Province, The Higher Educational Key Laboratory for Phosphorus Chemical Engineering of Yunnan Province, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming 650500, People’s Republic of China
Yang Meng
Yunnan Provincial Key Laboratory of Energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials, The International Joint Laboratory for Sustainable Polymers of Yunnan Province, The Higher Educational Key Laboratory for Phosphorus Chemical Engineering of Yunnan Province, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming 650500, People’s Republic of China
Jiangyu Zhang
Yunnan Provincial Key Laboratory of Energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials, The International Joint Laboratory for Sustainable Polymers of Yunnan Province, The Higher Educational Key Laboratory for Phosphorus Chemical Engineering of Yunnan Province, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming 650500, People’s Republic of China
Yuhui Xie
Yunnan Provincial Key Laboratory of Energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials, The International Joint Laboratory for Sustainable Polymers of Yunnan Province, The Higher Educational Key Laboratory for Phosphorus Chemical Engineering of Yunnan Province, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming 650500, People’s Republic of China
Hua Guo
Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an, Shaanxi 710072, People’s Republic of China
Mukun He
Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an, Shaanxi 710072, People’s Republic of China
Xuetao Shi
Shaanxi Key Laboratory of Macromolecular Science and Technology, School of Chemistry and Chemical Engineering, Northwestern Polytechnical University, Xi’an, Shaanxi 710072, People’s Republic of China
Yi Mei
Yunnan Provincial Key Laboratory of Energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials, The International Joint Laboratory for Sustainable Polymers of Yunnan Province, The Higher Educational Key Laboratory for Phosphorus Chemical Engineering of Yunnan Province, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming 650500, People’s Republic of China
Xinxin Sheng
Guangdong Provincial Key Laboratory of Functional Soft Condensed Matter, School of Materials and Energy, Guangdong University of Technology, Guangzhou 510006, People’s Republic of China
Delong Xie
Yunnan Provincial Key Laboratory of Energy Saving in Phosphorus Chemical Engineering and New Phosphorus Materials, The International Joint Laboratory for Sustainable Polymers of Yunnan Province, The Higher Educational Key Laboratory for Phosphorus Chemical Engineering of Yunnan Province, Faculty of Chemical Engineering, Kunming University of Science and Technology, Kunming 650500, People’s Republic of China

Corresponding Author: Delong Xie

cedlxie@kust.edu.cn

Nano-Micro Letters, Vol. 16 (2024), Article Number: 196

Abstract

Phase change materials (PCMs) offer a promising solution to address the challenges posed by intermittency and fluctuations in solar thermal utilization. However, for organic solid–liquid PCMs, issues such as leakage, low thermal conductivity, lack of efficient solar-thermal media, and flammability have constrained their broad applications. Herein, we present an innovative class of versatile composite phase change materials (CPCMs) developed through a facile and environmentally friendly synthesis approach, leveraging the inherent anisotropy and unidirectional porosity of wood aerogel (nanowood) to support polyethylene glycol (PEG). The wood modification process involves the incorporation of phytic acid (PA) and MXene hybrid structure through an evaporation-induced assembly method, which could impart non-leaking PEG filling while concurrently facilitating thermal conduction, light absorption, and flame-retardant. Consequently, the as-prepared wood-based CPCMs showcase enhanced thermal conductivity (0.82 W m−1 K−1, about 4.6 times than PEG) as well as high latent heat of 135.5 kJ kg−1 (91.5% encapsulation) with thermal durability and stability throughout at least 200 heating and cooling cycles, featuring dramatic solar-thermal conversion efficiency up to 98.58%. In addition, with the synergistic effect of phytic acid and MXene, the flame-retardant performance of the CPCMs has been significantly enhanced, showing a self-extinguishing behavior. Moreover, the excellent electromagnetic shielding of 44.45 dB was endowed to the CPCMs, relieving contemporary health hazards associated with electromagnetic waves. Overall, we capitalize on the exquisite wood cell structure with unidirectional transport inherent in the development of multifunctional CPCMs, showcasing the operational principle through a proof-of-concept prototype system.


Highlights:
1 An innovative class of versatile form-stable composite phase change materials (CPCMs) was fruitfully exploited, featuring MXene/phytic acid hybrid depositing on non-carbonized wood as a robust support.
2 The wood-based CPCMs showcase enhanced thermal conductivity of 0.82 W m−1 K−1 (4.6 times than polyethylene glycol) as well as high latent heat of 135.5 kJ kg−1 (91.5% encapsulation) with thermal durability and stability throughout at least 200 heating and cooling cycles.
3 The wood-based CPCMs have good solar-thermal-electricity conversion, flame-retardant, and electromagnetic shielding properties.

Keywords

Wood PCMs MXene Solar thermal storage and conversion Flame-retardant Electromagnetic shielding
Chen, Yuhui, Yang Meng, Jiangyu Zhang, Yuhui Xie, Hua Guo, Mukun He, Xuetao Shi, Yi Mei, Xinxin Sheng, and Delong Xie. 2024. “Leakage Proof, Flame-Retardant, and Electromagnetic Shield Wood Morphology Genetic Composite Phase Change Materials for Solar Thermal Energy Harvesting”. Nano-Micro Letters 16 (May):196. https://doi.org/10.1007/s40820-024-01414-4.
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