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Vol. 17 (2025)

Engineering Bipolar Doping in a Janus Dual-Atom Catalyst for Photo-Enhanced Rechargeable Zn-Air Battery

https://doi.org/10.1007/s40820-025-01707-2
Ning Liu
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Yinwu Li
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Wencai Liu
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Zhanhao Liang
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Bin Liao
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Fang Yang
Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education, Key Laboratory of High‑Performance Polymer‑Based Composites of Guangdong Province, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Ming Zhao
School of Materials Science and Engineering, Suzhou University of Science and Technology, Suzhou 215009, People’s Republic of China
Bo Yan
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Xuchun Gui
State Key Laboratory of Optoelectronic Materials and Technologies, School of Electronics and Information Technology, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Hong Bin Yang
School of Materials Science and Engineering, Suzhou University of Science and Technology, Suzhou 215009, People’s Republic of China
Dingshan Yu
Key Laboratory for Polymeric Composite and Functional Materials of Ministry of Education, Key Laboratory of High‑Performance Polymer‑Based Composites of Guangdong Province, School of Chemistry, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Zhiping Zeng
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China
Guowei Yang
State Key Laboratory of Optoelectronic Materials, School of Materials Science and Engineering, Sun Yat-Sen University, Guangzhou 510275, People’s Republic of China

Corresponding Author: Zhiping Zeng

zzhip8@mail.sysu.edu.cn

Nano-Micro Letters, Vol. 17 (2025), Article Number: 203

Abstract

Harnessing solar energy to enhance the rechargeable zinc–air batteries (RZABs) performance is a promising avenue toward sustainable energy storage and conversion. Simultaneously enhancing light-absorption capacity and carrier separation efficiency in nanomaterials, as well as improving electrical conductivity and configuration for electrocatalysis, presents a formidable challenge due to inherent trade-offs and interdependencies. Here, we have developed a Janus dual-atom catalyst (JDAC) with bifunctional centers for efficient charge separation and electrocatalytic performance through a bipolar doping strategy. The in situ X-ray absorption near-edge structure and Raman spectroscopy analyses demonstrated that the Ni and Fe centers in JDAC not only function as effective sites for oxygen evolution reaction and oxygen reduction reaction, respectively, but also serve as efficient hole and electron enrichment sites, effectively suppressing photoelectron recombination while enhancing photocurrent generation. As a result, the assembled JDAC-based light-assisted RZABs exhibited extraordinary stability at large current densities. This work delivers pivotal insight to design Janus dual-atom catalysts that efficiently convert solar energy into electric and chemical energy.


Highlights:
1 Janus dual-atom catalyst (JDAC) with bifunctional centers was synthesized via a single-step bipolar doping strategy to promote efficient charge separation and superior electrocatalytic performance.
2 The in situ X-ray absorption near-edge structure and Raman spectroscopy analyses demonstrated that Ni and Fe centers in JDAC function as effective sites for oxygen evolution reaction and oxygen reduction reaction, and effectively suppress photoelectron recombination while enhancing photocurrent generation.
3 The assembled JDAC-based light-assisted rechargeable zinc–air batteries exhibited extraordinary stability at large current densities (300 cycles at 50 mA cm−2, and 6000 cycles at 10 mA cm−2 under light illumination).

Keywords

Janus dual-atom catalyst Bifunctional center Bipolar doping Oxygen redox reaction Fuel cell
Liu, Ning, Yinwu Li, Wencai Liu, Zhanhao Liang, Bin Liao, Fang Yang, Ming Zhao, Bo Yan, Xuchun Gui, Hong Bin Yang, Dingshan Yu, Zhiping Zeng, and Guowei Yang. 2025. “Engineering Bipolar Doping in a Janus Dual-Atom Catalyst for Photo-Enhanced Rechargeable Zn-Air Battery”. Nano-Micro Letters 17 (March):203. https://doi.org/10.1007/s40820-025-01707-2.
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