Issue

Vol. 17 (2025)

Recent Advances in Wide-Range Temperature Metal-CO2 Batteries: A Mini Review

https://doi.org/10.1007/s40820-024-01607-x
Xuejing Zhang
School of Environmental and Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, People’s Republic of China
Ning Zhao
Engineering Research Center of Energy Storage Materials and Devices, Ministry of Education, School of Chemistry, Xi’an Jiaotong University, Xi’an 710049, People’s Republic of China
Hanqi Zhang
Engineering Research Center of Energy Storage Materials and Devices, Ministry of Education, School of Chemistry, Xi’an Jiaotong University, Xi’an 710049, People’s Republic of China
Yiming Fan
State Key Laboratory for Strength and Vibration of Mechanical Structures, Xi’an Jiaotong University, Xi’an 710049, People’s Republic of China
Feng Jin
State Key Laboratory for Strength and Vibration of Mechanical Structures, Xi’an Jiaotong University, Xi’an 710049, People’s Republic of China
Chunsheng Li
Key Laboratory of Advanced Electrode Materials for Novel Solar Cells for Petroleum and Chemical Industry of China, School of Chemistry and Life Sciences, Suzhou University of Science and Technology, Suzhou 215009, People’s Republic of China
Yan Sun
Key Laboratory of Advanced Electrode Materials for Novel Solar Cells for Petroleum and Chemical Industry of China, School of Chemistry and Life Sciences, Suzhou University of Science and Technology, Suzhou 215009, People’s Republic of China
Jiaqi Wang
Department of Chemistry and Biochemistry, Northern Illinois University, DeKalb, IL 60115, USA
Ming Chen
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou 225002, People’s Republic of China
Xiaofei Hu
Engineering Research Center of Energy Storage Materials and Devices, Ministry of Education, School of Chemistry, Xi’an Jiaotong University, Xi’an 710049, People’s Republic of China

Corresponding Author: Xiaofei Hu

xiaofei.hu@xjtu.edu.cn

Nano-Micro Letters, Vol. 17 (2025), Article Number: 99

Abstract

The metal–carbon dioxide batteries, emerging as high-energy–density energy storage devices, enable direct CO2 utilization, offering promising prospects for CO2 capture and utilization, energy conversion, and storage. However, the electrochemical performance of M-CO2 batteries faces significant challenges, particularly at extreme temperatures. Issues such as high overpotential, poor charge reversibility, and cycling capacity decay arise from complex reaction interfaces, sluggish oxidation kinetics, inefficient catalysts, dendrite growth, and unstable electrolytes. Despite significant advancements at room temperature, limited research has focused on the performance of M-CO2 batteries across a wide-temperature range. This review examines the effects of low and high temperatures on M-CO2 battery components and their reaction mechanism, as well as the advancements made in extending operational ranges from room temperature to extremely low and high temperatures. It discusses strategies to enhance electrochemical performance at extreme temperatures and outlines opportunities, challenges, and future directions for the development of M-CO2 batteries.


Highlights:
1 This review provides a comprehensive overview of the current research progress on metal–carbon dioxide (M-CO2) batteries across a broad temperature range (from room temperature to low/high temperatures).
2 The challenges encountered by M-CO2 batteries under extreme low- and high-temperature conditions thoroughly discussed, along with strategies to address these challenges.
3 The potential application scenarios and future directions of M-CO2 batteries across a broad temperature range are highlighted.

Keywords

M-CO2 batteries Wide-range temperature Electrolytes Interfaces Electrode reactions
Zhang, Xuejing, Ning Zhao, Hanqi Zhang, Yiming Fan, Feng Jin, Chunsheng Li, Yan Sun, Jiaqi Wang, Ming Chen, and Xiaofei Hu. 2024. “Recent Advances in Wide-Range Temperature Metal-CO2 Batteries: A Mini Review”. Nano-Micro Letters 17 (December):99. https://doi.org/10.1007/s40820-024-01607-x.
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