Issue

Vol. 19 (2027)

Rational Design of Covalent Organic Frameworks for Oxygen Electrocatalysis: Recent Advances and Mechanistic Insights

https://doi.org/10.1007/s40820-026-02281-x
Xinyan Zhang
Jiangsu Key Laboratory of Electrochemical Energy Storage Technologies, College of Material Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, People’s Republic of China
Ting Chen
Jiangsu Key Laboratory of Electrochemical Energy Storage Technologies, College of Material Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, People’s Republic of China
Zhengping Chen
Jiangsu Key Laboratory of Electrochemical Energy Storage Technologies, College of Material Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, People’s Republic of China
Gao Chen
Jiangsu Key Laboratory of New Energy Devices and Interface Science, School of Chemistry and Materials Science, Nanjing University of Information Science and Technology), Nanjing University of Information Science and Technology, Nanjing 210044, People’s Republic of China
Yanping Zhu
Jiangsu Key Laboratory of Electrochemical Energy Storage Technologies, College of Material Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, People’s Republic of China
Xiaogang Zhang
Jiangsu Key Laboratory of Electrochemical Energy Storage Technologies, College of Material Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, People’s Republic of China

Corresponding Author: Yanping Zhu

yanping.zhu@nuaa.edu.cn

Nano-Micro Letters, Vol. 19 (2027), Article Number: 14

Abstract

Due to the excessive consumption of fossil fuels and the increasingly severe global environment, the world urgently needs to develop new clean and renewable energy sources. However, these energy sources have intermittency and instability, so it is necessary to vigorously develop efficient and large-scale energy conversion and storage technologies such as fuel cells, water electrolyzers, and metal–air batteries based on the core reactions of oxygen evolution reaction and oxygen reduction reaction. Because of their excellent molecular designability and structural tunability, covalent organic frameworks (COFs) show great potential for applications in this field. In this review, we first classify COF-based electrocatalysts based on the nature of active sites. Subsequently, strategies including structural design and functional synthesis for improving performance of COF-based electrocatalysts in the field of oxygen catalysis are systematically reviewed. Importantly, mechanism discussion of the performance improvement is highlighted. Finally, we put forward prospects for the future research directions, challenges, and development opportunities in this field. This review aims to provide guidance for the development of high-performance COF-based electrocatalysts through critical analysis of existing research, revealing the correlation between material design and mechanism for performance improvement.


Highlights:
1 Comprehensive classification of covalent organic frameworks (COFs)-based electrocatalysts based on the nature of active sites.
2 Systematic review of structural design and functional synthesis strategies for enhancing oxygen electrocatalysis.
3 In-depth mechanistic insights into performance improvement and future perspectives for COF-based oxygen electrocatalysts.

Keywords

Covalent organic frameworks Electrocatalysts Oxygen reduction reaction Oxygen evolution reaction
Zhang, Xinyan, Ting Chen, Zhengping Chen, Gao Chen, Yanping Zhu, and Xiaogang Zhang. 2026. “Rational Design of Covalent Organic Frameworks for Oxygen Electrocatalysis: Recent Advances and Mechanistic Insights”. Nano-Micro Letters 19 (July):14. https://doi.org/10.1007/s40820-026-02281-x.
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