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Vol. 15 (2023)

Recent Advances in Structural Optimization and Surface Modification on Current Collectors for High-Performance Zinc Anode: Principles, Strategies, and Challenges

https://doi.org/10.1007/s40820-023-01177-4
Yuxin Gong
MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, Heilongjiang, People’s Republic of China
Bo Wang
MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, Heilongjiang, People’s Republic of China
Huaizheng Ren
MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, Heilongjiang, People’s Republic of China
Deyu Li
MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, Heilongjiang, People’s Republic of China
Dianlong Wang
MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, Heilongjiang, People’s Republic of China
Huakun Liu
Institute of Energy Material Science, University of Shanghai for Science and Technology, Shanghai 200093, People’s Republic of China
Shixue Dou
Institute of Energy Material Science, University of Shanghai for Science and Technology, Shanghai 200093, People’s Republic of China

Nano-Micro Letters, Vol. 15 (2023), Article Number: 208

Abstract

The last several years have witnessed the prosperous development of zinc-ion batteries (ZIBs), which are considered as a promising competitor of energy storage systems thanks to their low cost and high safety. However, the reversibility and availability of this system are blighted by problems such as uncontrollable dendritic growth, hydrogen evolution, and corrosion passivation on anode side. A functionally and structurally well-designed anode current collectors (CCs) is believed as a viable solution for those problems, with a lack of summarization according to its working mechanisms. Herein, this review focuses on the challenges of zinc anode and the mechanisms of modified anode CCs, which can be divided into zincophilic modification, structural design, and steering the preferred crystal facet orientation. The possible prospects and directions on zinc anode research and design are proposed at the end to hopefully promote the practical application of ZIBs.


Highlights:
1 The mechanisms of the surface modification and structure design of zinc anode current collectors were summarized.
2 The recent advances of high-performance zinc anode current collectors were reviewed and categorized according to their working mechanisms.
3 The possible prospects and directions of zinc anode research were discussed.

Keywords

Zinc anodes Current collectors Surface modification Structural design Crystal facet orientation
Gong, Yuxin, Bo Wang, Huaizheng Ren, Deyu Li, Dianlong Wang, Huakun Liu, and Shixue Dou. 2023. “Recent Advances in Structural Optimization and Surface Modification on Current Collectors for High-Performance Zinc Anode: Principles, Strategies, and Challenges”. Nano-Micro Letters 15 (August):208. https://doi.org/10.1007/s40820-023-01177-4.
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